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Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.

Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.

期刊: Marine drugs 日期: 2026-05-30 PMID: 42346779 DOI: 10.3390/md24060193 浏览: 22
作者: Leshchenko EV, Borkunov GV, Antonov AS, Chingizova EA, Berdyshev DV, Solovova MA, Popov RS, Sayankina KA, Khudyakova YV, Baldaev SN
EV, L., GV, B., AS, A., EA, C., DV, B., MA, S., RS, P., KA, S., YV, K., & SN, B. (2026). Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.. Marine drugs. https://doi.org/10.3390/md24060193
EV L, GV B, AS A, EA C, DV B, MA S, et al. Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.. Marine drugs. 2026; doi: 10.3390/md24060193
EV L, GV B, AS A, et al. Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.[J]. Marine drugs. 2026. DOI: 10.3390/md24060193.
@article{ev2026,
  author = {Leshchenko EV and Borkunov GV and Antonov AS and Chingizova EA and Berdyshev DV and Solovova MA and Popov RS and Sayankina KA and Khudyakova YV and Baldaev SN},
  title = {Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.},
  journal = {Marine drugs},
  year = {2026},
  doi = {10.3390/md24060193},
  note = {PMID: 42346779},
}
TY  - JOUR
AU  - Leshchenko EV
AU  - Borkunov GV
AU  - Antonov AS
AU  - Chingizova EA
AU  - Berdyshev DV
AU  - Solovova MA
AU  - Popov RS
AU  - Sayankina KA
AU  - Khudyakova YV
AU  - Baldaev SN
TI  - Discovery of New Zosteropenillines from the Seagrass-Derived Fungus Penicillium yezoense KMM 4679 by OSMAC Strategy.
T2  - Marine drugs
PY  - 2026
DO  - 10.3390/md24060193
AN  - PMID:42346779
ER  - 

摘要

Thirteen new decaline polyketides, namely, zosteropenillines T-W (1-4), 8-hydroxypallidopenilline A (5), 13-epi-zosteropenilline P (6), 11-epi-zosteropenilline N (7), 15-hydroxyzosteropenilline M (8), 8-hydroxyzosteropenilline M (9), 11-epi-zosteropenilline M (10), and zosteropenillines X-Z (11-13), along with 17 known related compounds (14-30) were isolated from the ethyl acetate extract of the marine-derived fungus Penicillium yezoense KMM 4679 cultivated on MgCl2-containing nutrient medium. The structures of the isolated compounds were established based on spectroscopic methods. The absolute configurations of zosteropenillines T (1) and V (3) were determined using time-dependent density functional theory (TD-DFT) calculations of the ECD spectra. X-ray diffraction analysis data were obtained for the known zosteropenilline S (28). A biogenetic pathway for 1-13 was proposed. The effects of the compounds on Staphylococcus aureus and Candida albicans growth and biofilm formation were observed. Zosteropenillines U (2), Y (12) and Z (13) with higher activity against C. albicans biofilms were nontoxic for normal cardiomyocyte H9c2 cells, making them promising anti-candidal agents. Moreover, zosteropenillines U and Y demonstrated cardioprotective effects in acute ischemia/reperfusion and CoCl2-mimicking hypoxia in vitro models.

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