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In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.

In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.

期刊: Scientific reports 日期: 2026-07-23 PMID: 42493523 DOI: 10.1038/s41598-026-56505-6 浏览: 19
作者: Elkotamy MS, Elgohary MK, Alkotami AS, Eldesouki MM, Elsayed ZM, Mattar AA, Abo-Ashour MF, Tawfik HO, Eldehna WM, Abdel-Aziz HA
MS, E., MK, E., AS, A., MM, E., ZM, E., AA, M., MF, A.A., HO, T., WM, E., & HA, A.A. (2026). In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.. Scientific reports. https://doi.org/10.1038/s41598-026-56505-6
MS E, MK E, AS A, MM E, ZM E, AA M, et al. In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.. Scientific reports. 2026; doi: 10.1038/s41598-026-56505-6
MS E, MK E, AS A, et al. In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.[J]. Scientific reports. 2026. DOI: 10.1038/s41598-026-56505-6.
@article{ms2026,
  author = {Elkotamy MS and Elgohary MK and Alkotami AS and Eldesouki MM and Elsayed ZM and Mattar AA and Abo-Ashour MF and Tawfik HO and Eldehna WM and Abdel-Aziz HA},
  title = {In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.},
  journal = {Scientific reports},
  year = {2026},
  doi = {10.1038/s41598-026-56505-6},
  note = {PMID: 42493523},
}
TY  - JOUR
AU  - Elkotamy MS
AU  - Elgohary MK
AU  - Alkotami AS
AU  - Eldesouki MM
AU  - Elsayed ZM
AU  - Mattar AA
AU  - Abo-Ashour MF
AU  - Tawfik HO
AU  - Eldehna WM
AU  - Abdel-Aziz HA
TI  - In silico pipeline for GSK 3β inhibitor discovery in Alzheimer's disease using pharmacophore screening, docking, ADME filtering, and MD validation.
T2  - Scientific reports
PY  - 2026
DO  - 10.1038/s41598-026-56505-6
AN  - PMID:42493523
ER  - 

摘要

Glycogen synthase kinase-3β (GSK-3β) is a key therapeutic target for Alzheimer's disease, but identifying safe, brain-penetrant inhibitors remains difficult. This study aimed to discover novel CNS-active GSK-3β inhibitors using a rigorous multi-tier computational pipeline. The workflow combined ligand-based and structure-based pharmacophore modeling, virtual screening of the ZINCPharmer database, AutoDock Vina docking, ADME and blood-brain barrier (BBB) filtering with SwissADME, toxicity prediction using ProTox-3.0, and validation by 100-ns molecular dynamics simulations with MM/GBSA and MM/PBSA free energy calculations. Pharmacophore screening with a ≤ 1.0 Å RMSD cutoff identified 1,085 ligand-based and 36 structure-based hits. After docking and developability filtering, two BBB-permeant candidates were prioritized: SB1, a structure-based hit (predicted LD50 = 2500 mg/kg, toxicity class 5), and LB1, a ligand-based hit (predicted LD50 = 521 mg/kg, toxicity class 4). Molecular dynamics confirmed stable binding for both compounds. MM/GBSA analysis showed favorable binding free energies for SB1 (-27.68 kcal/mol) and LB1 (-25.74 kcal/mol), both surpassing the co-crystallized reference (-8.75 kcal/mol). These findings identify SB1 and LB1 as promising, safe, and brain-penetrant GSK-3β lead compounds for experimental validation in Alzheimer's disease.

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